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This is a Experimental Study study.

Direct Access to Aminocyclopentenones through Rh‐Catalyzed Cascade Wolff Rearrangement and Decarbonylative Amination

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The cascade reaction provides efficient access to 2-aminocyclopentenones with yields ranging from 71% to 90%.
Utilizing a Rh catalyst, the reaction proceeds through Wolff rearrangement and subsequent decarbonylative amination.
A wide range of substrates can undergo this mild reaction, highlighting its versatility.
The proposed sequence contributes to a practical method for constructing important aminocyclopentenone structures.

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This method demonstrates the efficient formation of aminocyclopentenones through Wolff rearrangement and decarbonylative amination.

Gao et al. (2025) studied this question.

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