In the race toward increasingly high-performance trace-molecule sensors, one of the most significant steps forward in the last decade for photoacoustic sensors was their combination with high-finesse optical cavities. Validated with different configurations, this technique demonstrated enhanced sensitivities below the part-per-trillion level (ppt) and record dynamic ranges. Here we present our advanced cantilever-based photoacoustic setup, based on a custom-made silicon cantilever embedded in a doubly-resonant configuration. The combination of a high-quality-factor acoustic resonator and a high-finesse optical cavity allows a final sensitivity enhancement by several orders of magnitude. The sensor was tested on strong N₂O transitions around 4.5 μm wavelength with a continuous-wave quantum cascade laser.
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Pelini et al. (2024) studied this question.
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