High-level computations and experiments show that DDQ oxidations alter electron transfer reactivity, indicating a need to rethink established paradigms.
High-level computations and experiments reveal that DDQ–alkene oxidations operate on an ACET–AdE2 continuum, providing the first experimental validation of ACET and redefining electron-transfer reactivity beyond the SET paradigm.
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Ma et al. (2025) studied this question.
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