MOFs with Hydrazide and 3-Amino-1,2,4-oxadiazole-Substituted Hydroxytetrazole as Novel Nitrogen-Rich Ligands: A New Type of Energetic Materials for Ammonium Perchlorate Decomposition Catalysis

Feng Yang; Zhiwei He; Rongzheng Zhang; Quan Wang

doi:10.1039/d5ce01001b

January 1, 2026CrystEngComm

MOFs with Hydrazide and 3-Amino-1,2,4-oxadiazole-Substituted Hydroxytetrazole as Novel Nitrogen-Rich Ligands: A New Type of Energetic Materials for Ammonium Perchlorate Decomposition Catalysis

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Key Points

The research aims to create metal-organic frameworks (MOFs) that enhance the decomposition of ammonium perchlorate (AP) using novel ligands.
Synthesize energetic MOFs using hydrazide and 3-amino-1,2,4-oxadiazole-substituted hydroxytetrazole as ligands.
Test the catalytic activity of these MOFs for AP decomposition under controlled conditions.
Analyze the combustion efficiency of the newly developed materials.
The newly synthesized MOFs demonstrated improved catalytic performance for AP decomposition compared to traditional methods.
Enhanced decomposition rates were observed, indicating potential for better combustion efficiency.
The use of nitrogen-rich ligands successfully increased the energy release during AP combustion.

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Implication

Laboratory experiments develop new energetic materials to enhance ammonium perchlorate decomposition, indicating potential for improved combustion efficiency.

Abstract

To address the issue of insufficient combustion of ammonium perchlorate (AP), the development of energetic MOFs that facilitate the decomposition of AP has emerged as one of the primary focuses...

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Yang et al. (2026) studied this question.

synapsesocial.com/papers/69897996f0ec2af6756e74af https://doi.org/10.1039/d5ce01001b

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MOFs with Hydrazide and 3-Amino-1,2,4-oxadiazole-Substituted Hydroxytetrazole as Novel Nitrogen-Rich Ligands: A New Type of Energetic Materials for Ammonium Perchlorate Decomposition Catalysis

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MOFs with Hydrazide and 3-Amino-1,2,4-oxadiazole-Substituted Hydroxytetrazole as Novel Nitrogen-Rich Ligands: A New Type of Energetic Materials for Ammonium Perchlorate Decomposition Catalysis

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