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June 19, 2026ACS Catalysis

Tandem C−N Coupling for Acetamide Synthesis via Paired Electrolysis Using a Bifunctional Catalyst

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Authors

JLJin LiuMGMing‐Hao GuanXZXiao-Ya Zhou

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Overview

Randomized trial demonstrates efficient acetamide synthesis using paired electrolysis with a bifunctional catalyst.

Key Points

  • The aim is to improve the efficiency of amide synthesis via paired electrosynthesis using a bifunctional catalyst.
  • Integration of cathodic nitrite reduction (NO2 RR) and anodic ethanol oxidation (EOR) using a bifunctional NiCo2O4/NiCo-NCNT electrocatalyst.
  • In situ spectroscopic analysis to confirm the reaction mechanism.
  • Flow cell experiments conducted to assess yield and current densities.
  • Achieved amide synthesis yield of 815.47 μmol cm−2 h−1 in a flow cell.
  • Enabled gram-scale production at current densities up to 310 mA cm−2.
  • Synergistic reactions facilitated efficient C−N bond formation between CH3CHO and NH3/NH2OH.

Cite This Study

Liu et al. (2026) studied this question.

synapsesocial.com/papers/6a34dc0f65a5b0777af2c6e2https://doi.org/10.1021/acscatal.6c02963
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