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June 28, 2026Advanced Materials

Molecular Interfacial Engineering of Lithiophilic Protection Layer Realizing 600 Wh kg −1 Anode‐Free Lithium Metal Batteries

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Authors

YLYazhan LiangNSNing SongJCJ Y Chen

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Overview

Randomized trial demonstrates improved energy density in lithium metal batteries, highlighting scalable engineering strategies.

Key Points

  • The study aims to enhance the performance and safety of anode-free lithium metal batteries through molecular interface engineering.
  • Developed a self-assembled monolayer interface using 5-methyl-1H-tetrazole on copper foil surfaces.
  • Evaluated energy density and plating uniformity in anode-free lithium metal pouch cells with modified Cu foil.
  • Conducted tests using specific cathodes LiNi 0.8 Co 0.1 Mn 0.1 O 2 and LiNi 0.9 Co 0.05 Mn 0.05 O 2.
  • Achieved energy densities of 505.31 Wh kg total −1 and 605.96 Wh kg total −1 for pouch cells over 100 cycles.
  • Demonstrated improved lithium plating uniformity and reversibility due to the self-assembled monolayer.
  • Showed potential for large-scale production, indicating commercial applicability.

Cite This Study

Liang et al. (2026) studied this question.

synapsesocial.com/papers/6a40b9c461bb0a67205c5d68https://doi.org/10.1002/adma.73830
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