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Picosecond Raman spectra of adsorbed CN were obtained for the first time in the presence of extensive surface damage. The incident laser intensity was 40 times than previously reported. At this intensity, nonlinear Raman spectroscopy such as coherent anti-Stokes Raman scattering should be feasible without dependence on surface enhancement.
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Paddock et al. (1982) studied this question.
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