The preparation and evaluation of some interstitial compounds is described and their potential as high transition temperature superconductors discussed. An evaluation of transition temperature measurements of pseudo-binary and ternary interstitial alloys shows that no simple direct relationship exists between transition temperature and such quantities as valence electron-atom ratio, mass and lattice volume. However, the experimental data have been successfully systematized in terms of a general empirical model which appears capable of predicting the most promising materials for attaining high transition temperatures. Preliminary data demonstrate that a large number of alloyed interstitial compounds exhibit transition temperatures in the vicinity of 18^∘K.
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Pessall et al. (1966) studied this question.
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