Giant enhancement of the intrinsic spin Hall conductivity in β -tungsten via substitutional doping

This is the authors' abstract. We don't add key points for this paper.

A key challenge in manipulating the magnetization in heavy-metal/ferromagnetic bilayers via the spin-orbit torque is to identify materials that exhibit an efficient charge-to-spin current conversion. Ab initio electronic structure calculations reveal that the intrinsic spin Hall conductivity (SHC) for pristine β-W is about 60% larger than that of α-W. More importantly, we demonstrate that the SHC of β-W can be enhanced via Ta alloying. This is corroborated by spin Berry curvature calculations of W_1-xTaₓ (x~12.5%) alloys which show a giant enhancement of the spin Hall angle of up to ≈-0.5. The underlying mechanism is the synergistic behavior of the SHC and longitudinal conductivity with the Fermi level position. These findings not only pave the way for enhancing the intrinsic spin Hall effect in β-W, but also provide guidelines to exploit substitutional alloying to tailor the spin Hall effect in various materials.