Basic Theory of Electrical Double Layer Formation at Solid-Liquid and Solid-Solid Interfaces

Q: What does this research mean for the field?

A comprehensive understanding of electrical double layer (EDL) formation at solid-liquid and solid-solid interfaces, integrating classical models with modern molecular approaches, is fundamental for controlling interfacial reactions and designing next-generation electrochemical devices. Novelty: ClaimNovelty.SYNTHESIS. Consensus alignment: ConsensusAlignment.NEUTRAL.

Masahiro YAMAMOTO

doi:10.5796/denkikagaku.26-fe0306

September 4, 2026Denki KagakuOpen Access

Basic Theory of Electrical Double Layer Formation at Solid-Liquid and Solid-Solid Interfaces

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Key Points

To synthesize theoretical frameworks describing electrical double layer formation at solid-liquid and solid-solid interfaces to guide next-generation electrochemical device design.
Reviewed continuum electrostatic formulations, centered on the classical Gouy–Chapman–Stern model.
Surveyed molecular-scale and statistical thermodynamic models capturing microscopic ion and electron distributions.
Evaluated interfacial behaviors specific to solid electrolyte boundaries and nanoconfined spaces relevant to all-solid-state and lithium-ion batteries.
Modern statistical and molecular models overcome continuum limitations to characterize local charge accumulation and potential gradients at electrified interfaces.
Interfacial charge distributions in solid electrolytes and nanospaces deviate markedly from liquid electrolytes, directly dictating charge transfer kinetics and interface stability in solid-state devices.

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Implication

Narrative review outlines theoretical models of electrical double layer formation across interfaces, highlighting mechanisms to advance solid-state battery design.

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Masahiro YAMAMOTO (2026) studied this question.

synapsesocial.com/papers/6a9e8559c3034f961570d8e2 https://doi.org/10.5796/denkikagaku.26-fe0306

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Basic Theory of Electrical Double Layer Formation at Solid-Liquid and Solid-Solid Interfaces

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Basic Theory of Electrical Double Layer Formation at Solid-Liquid and Solid-Solid Interfaces

Key Points

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