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Cleavage of unstrained C−C bonds under mild, redox‐neutral conditions represents a challenging endeavor which is accomplished here in the context of a flexible, visible‐light‐mediated, γ‐functionalization of amines. In situ generated C‐centered radicals are harvested in the presence of Michael acceptors, thiols and alkyl halides to efficiently form new C(sp 3 )−C(sp 3 ), C(sp 3 )−H and C(sp 3 )−Br bonds, respectively.
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Shu et al. (2017) studied this question.
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