November 28, 2025Catalysis Science & Technology

Metal-ligand cooperative strategy of Zn-catalyst for multicomponent synthesis of highly substituted pyrazolines, pyrimidines, and quinolines: A combined experimental and DFT optimized study

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Demonstrates the efficacy of a Zn-catalyst for synthesizing N-heterocycles.
Key findings include the successful conversion of renewable primary alcohols to quinolines and more.
Experimental approach combined with DFT optimization highlights the feasibility of this method.
Supports the use of sustainable resources in chemical synthesis, showcasing renewable alcohols' potential.

Implication

Experimental and DFT analysis reveals a Zn-catalyst method for N-heterocycles synthesis, suggesting efficiency in renewable alcohol use.

Abstract

In this study, we disclose a Zn(II)- catalysed metal-ligand cooperative approach that converts renewable primary alcohols into highly substituted N-heterocycles via acceptor-less dehydrogenation. A well-defined Zn(II) complex, C1, supported by...

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Cite This Study

Kukreti et al. (2025) studied this question.

synapsesocial.com/papers/6928f126a65b730b9ea7a4c1 https://doi.org/10.1039/d5cy01110h

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Implication

Experimental and DFT analysis reveals a Zn-catalyst method for N-heterocycles synthesis, suggesting efficiency in renewable alcohol use.

Metal-ligand cooperative strategy of Zn-catalyst for multicomponent synthesis of highly substituted pyrazolines, pyrimidines, and quinolines: A combined experimental and DFT optimized study

Key Points

Implication

Abstract

Discussion

Cite This Study

Metal-ligand cooperative strategy of Zn-catalyst for multicomponent synthesis of highly substituted pyrazolines, pyrimidines, and quinolines: A combined experimental and DFT optimized study

Key Points

Implication

Abstract

Discussion

Cite This Study

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