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The electronic configuration and bonding in (PuO2)2+ are considered. The calculated energy levels can be correlated satisfactorily with the absorption spectrum of (PuO2)2+ in aqueous solution by a plausible choice of numerical parameters. The microwave resonance absorption and paramagnetic susceptibility are derived on the basis of the model, and are in good agreement with experimental results.
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Eisenstein et al. (1956) studied this question.
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